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Cloud Microphysics SOEE3410 : Lecture 6 Ken Carslaw Lecture 2 of a series of 5 on clouds and climate • Properties and distribution of clouds • Cloud microphysics and precipitation • Clouds and radiation • Clouds and climate: forced changes to clouds • Clouds and climate: cloud response to climate change Content of Lecture 6 • Drop formation – factors controlling drop number and size • Rain formation – what is needed? • The ice phase ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1 Recommended Reading for This Lecture • A Short Course on Cloud Physics, R. R. Rogers and M. K. Yau, 3rd ed., Butterworth-Heinemann – Some very readable chapters – Physics L-0 Rog (Reference, short, long) • Several cloud physics books in the library worth flicking through ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1 What is Cloud Microphysics? • Properties of a cloud on the micro-scale (i.e., micrometres) • Includes droplet concentrations, sizes, ice crystal formation, droplet-droplet interactions, rain drop formation, etc. ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1 Microphysics and Climate • Cloud drop number (CDN) influences cloud albedo (next lecture) – Ist indirect effect of aerosols on climate • CDN/size influences precipitation efficiency (and therefore cloud lifetime/distribution and cloud fraction) – 2nd indirect effect of aerosols on climate • Ice formation affects latent heat release, precipitation intensity, cirrus properties,etc. ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1 Microphysical Processes • Drop formation – What determines the number and size of drops? • Drop spectrum broadening (collision and coalescence) – How do some drops grow to precipitation-sized particles in the time available? • Ice formation • Ice phase processes (riming, accretion, etc) ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1 Condensation Nuclei Starting Point for Drop Formation • Droplets form by condensation of water vapour on aerosol particles (condensation nuclei, CN) at very close to 100% RH • Without CN, humidities of >300% are required for drop formation • Droplets form on some (a subset of) CN – Cloud Condensation Nuclei (CCN) • CN are composed of – Salt particles from sea spray – Natural material (inorganic and organic mixtures) – Human pollution (sulphuric acid particles, etc) ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1 Cloud Formation Either: • Air rises and cools to saturation (100% RH) and then supersaturation (>100% RH) – Adiabatic expansion • Air cools by radiative energy loss or advection over a cold surface (fogs) ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1 Increase in humidity in a rising air parcel pw % RH 100. 0 pw Partial pressure of water in the air Saturation vapour pressure over pure water water pressure 100% RH line >100% RH above the line Droplets form Air initially at 70% RH Air rises, cools, RH increases 100% RH (saturation, dew point) Droplets grow, remove water vapour temperature ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1 Droplet “activation” sea salt ammonium sulphate >100% RH (supersaturation) needed to form drops • Small particles require higher humidities because surface tension of small droplets increases the pressure of water vapour over their surface • Consequence: droplets form on large particles first ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1 Droplet “activation” Typically 1000-10000 cm-3 Typically 100-1000 cm-3 growth maximum supersaturation in cloud equates to minimum radius of activation ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1 Factors affecting droplet number • Aerosol particle size } – larger particles activate at lower humidities • Particle chemical composition – Some substances are more ‘hygroscopic’ Human activities affect these • Aerosol particle number concentration – Simple • Cloud-scale updraught speed – Higher speed = more drops ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1 Droplet number vs. aerosol size and number • Fixed updraught speed See Pringle et al., ACP, http://tinyurl.com/39rwk3r log(N) Solid contours = CDN; colours = aerosol mass (mg m-3) ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics Diameter 1 Droplet Evolution Above Cloud Base updraught = 2.0 ms-1 Height above cloud base (m) updraught = 0.5 ms-1 80 60 Decreasing supersat’n 80 as droplets grow, suppresses 60 new droplets 80 80 60 60 40 40 40 40 20 20 20 20 0 0 0 0 0 0.4 0.6 Supersaturation (%) 0 200 400 0 2 4 6 Drop conc’n (cm-3) Ave’ radius (mm) (S = %RH-100) ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 0 0.1 0.2 Liquid water content (g m-3) 1 Diffusional Droplet Growth Droplets grow by diffusion of water vapour dr S r dt const (S = %RH-100) Radius time 1 2.4 s 2 130 s 4 1000 s 10 2700 s 20 2.4 hr 30 4.9 hr 40 12.4 hr transition drop r=50, V=27 typical drop r=10, V=1 NaCl particle (10-14 g mass); initial radius = 0.75 micron; RH = 100.05%; p = 900 mb; T = 273 K large drop r=50, V=27 . typical CN r=0.1, V=10-4 typical raindrop: r=1000, V=650 ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1 Diffusional Droplet Growth dr S r dt const • Leads to narrowing of droplet size distribution, but not observed Diffusion only Observed • Possible reasons: Ndrop Ndrop – Giant CN – Supersaturation fluctuations – Mixing cloud top cloud base Diameter ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics cloud base cloud top Diameter 1 Definition of “Precipitation-Sized” Droplet • How big must a droplet be before it can be considered a “raindrop” Initial radius Distance fallen 1 mm 2.0 mm 3 mm 0.17 mm 10 mm 2.1 cm 30 mm 1.69 m 0.1 mm 208 m 0.15 mm 1.05 km Distance a drop falls before evaporating. Assumes isothermal atmosphere with T=280 K, RH=80% Definition of a drizzle drop ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1 “Warm Rain” Formation • Rain formation without ice phase • Additional process needed to grow droplets to precipitation size • Collision and coalescence – Two processes: collision rate and coalescence rate Narrow distributions not very efficient for collision Some large drops initiate collisioncoalescence ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1 Collision and Coalescence Rates “wake” effects Almost all collisions result in coalescence Collision-Coalescence efficiency reduced because small drops are swept round the larger one Coalescence very inefficient below about 20 mm Therefore droplet distribution broadening needed ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1 Droplet Evolution with CollisionCoalescence 30 25 20 15 10 5 0 10-3 10-2 10-1 100 Radius (cm) 10 mm ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1 Summary of “Warm Cloud” Microphysics • Precipitation is favoured in clouds with – – – – Large liquid water content (i.e., deep cumulus) Broad drop spectrum Large drops (must be larger than ~20 mm) Large vertical extent (=long growth/collision times) ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1 Precipitation Formation Through Ice Processes Ice forms on ice nuclei (IN) • Silicates (soil dust, etc.) • Clays • Fungal spores • Combustion particles (soot, etc.) • Other industrial material ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1 Ice formation Processes Water drops readily supercool below 0oC without freezing See http://www.youtube.com/watch?v=0JtBZGXd5zo Between –10 oC and –39 oC Result = very few crystals Contact nucleation freezing Immersion freezing (Rate proportional to drop volume) Deposition nucleation (reverse sublimation) Below –39 oC Result = complete freezing Homogeneous of all drops freezing ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1 The Growth Advantage of Ice Crystals At –20 oC at 100% RH Sice = 24% Air is Marginally supersaturated with respect to liquid water in a rising cloud thermal Compare with typical Sliq = 0.05-0.5% ! Highly supersaturated with respect to ice Few crystals grow at expense of drops Subsequent growth from accretion and aggregation ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1 Atmospheric Ice Nuclei Concentrations ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1 Effect of Freezing on Cloud Development • Intensification of rain • Release of latent heat aloft (giving further buoyancy) ENVI3410 : Coupled Ocean & Atmosphere Climate Dynamics 1